Roggenart has a few locations, but they can get pretty busy.

It's not really a coffee shop, but Bonheur Patisserie & Deli always has a ton of variety and they sell coffee in addition to the baked goods and sandwiches. We've pretty much always had good experiences there.

Edit: Also, Decadent is towards Laurel and has a bunch of coffee options in addition to baked goods. I think they sell Irish coffees there too.