Shawn and Gus from Psych

Literal perfection in a duo.

It isn't a pair of characters but I love Danny Mcbride and Walton Goggins together. Vice Principals and the Gemstones are sheer chaos and hilarity.

Bob Mortimer and Paul Whitehouse from Mortimer & Whitehouse Gone Fishing

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Richard Richard & Edward Elizabeth Hitler

Scooby and Shaggy

Ralph Kramden and Ed Norton.

Vorenus and Pullo

Arya and Sandor Clegane from GOT